It looks to me (not being an 68k expert) that only the first word is considered the "opcode": the second word just selects what "D" registers are used for the CAS operation. Normally one would expect the zero bits to be completely ignored in that case, since they don't have any role in the instruction.
But maybe on the 68030 in this case, the bits must be zero even if they have no documented use, because there is hardwired logic for another instruction that is activated by those bits being set, somewhat like the 6502 illegal opcodes?
It's reminiscent of ARM, but the relevant part is that the CAS instruction's second word bits 5:0 look like a "modrm" (to use the x86 terminology) where the officially documented values select only Dn, but the undocumented variant would correspond to (d16,An). At least, that's my theory for why A1 gets modified.
It also appears that I may not have been the first one to discover that something odd was going on with that bit, causing it to use A0-A7 (with weird results) instead of D0-D7:
But maybe on the 68030 in this case, the bits must be zero even if they have no documented use, because there is hardwired logic for another instruction that is activated by those bits being set, somewhat like the 6502 illegal opcodes?