James narrating Edgar Allan Poe's The Raven in the very first Simpsons Treehouse of Horror episode (2x03), to the backdrop of the quirky and artistic early-Simpsons animation, was such a wonderful union of beautiful cross-generational zeitgeist.
Here's a different reading by him of The Raven (not the one from The Simpsons): https://www.youtube.com/watch?v=sXU3RfB7308 — he chooses to almost ignore the meaning and stick to a recitation, which is great: his voice perfectly brings out the poem's cadence and assonance.
Other readings of The Raven, for comparison: Christopher Walken [1], Vincent Price [2], Christopher Lee (build-up in intensity, unfortunately some background music) [3], Basil Rathbone (the opposite of James Earl Jones: in places almost like prose) [4]
And still, for me, the best reading of that! There are many renditions out there by some very accomplished actors but I've never heard or seen a better one.
My Simpsons memory of him is him coming up from the clouds as Mustafa, Darth Vader, and himself saying "This is CNN". But TIL it wasn't him but Harry Shearer doing an impression.
